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For the most widely used hole transport layer (HTL) of 2,2',7,7'-Tetrakis[N,N-di(4-methoxyphenyl)amino]-9,9'-spirobifluorene (Spiro-OMeTAD), it would undergo morphology change via outgassing or crystallization under heat, leading to the formation of voids and failure of separation (Fig

It also helps to understand why the three arms were combined in the first place